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More importantly, ternary reactivity ratios are never determined using ternary experimental data, and differences in the system make it imprudent to use binary and ternary reactivity ratios interchangeably. Using inappropriate reactivity ratios may affect the model performance for predicting terpolymer composition (and sequence length characteristics, since these also depend on reactivity ratio values) and the determination of other terpolymerization characteristics (such as the azeotropic point).
Despite these risks, all studies performed previously have employed binary reactivity ratios directly in terpolymer models. Parameter estimation and the implementation of the design of experiments strategy are demonstrated, and the reactivity ratio estimates are analyzed in terms of both precision and accuracy.
Finally, reactivity ratio values based on optimally selected experiments are suggested.